Also try this
Enumerable
.Range('A', 'Z' - 'A' + 1)
.ToList()
.ForEach(i => Console.WriteLine((Char)i));
Another Way
Enumerable
.Range(0, 26)
.ToList()
.ForEach(i => Console.WriteLine(Convert.ToChar(i + 65 + 0)));
For generating Small letters write
i + 65 + 32
Another way
"ABCDEFGHIJKLMNOPQRSTUVWXYZ"
.ToCharArray()
.ToList()
.ForEach(i => Console.WriteLine(i));